When you live in nature, you just do as you feel. No reference, no efficiency, it's freeing; and that's a feeling you rarely get in society.
The closest you can currently get to "doing as you feel", involves moving to Europe and becoming dependent on the socialist state. You can live for free in a flat forever, never have to work, get free health care for every booboo, just hang out all day surrounded by people who do the same thing. I would say this is currently the state of the art in living an unnatural life. And as a result, you might end up being miserable.
But I do sort of understand what you mean; our brains were built for living in natural environments. These impose fairly random and complex constraints, with stress coming in big but short-lived peaks and real family being constantly around.
Living in a concrete jungle and having constant low level stress, doing and eating the exact same things every day, taking pills for every little ill is a recipe for alienation and early death.
But I don't intend for this to become a political discussion. To me, this is just an effective example of how "doing what you feel like" can be very different from living in nature or in a natural state and being happy.
(It worked out okay, but I didn't realize I should have had a wheelchair on hand recently when I picked someone up from a relatively straightforward orthopedic surgery)
Contrast with the often hyper competitive social/city environment.
Walking down the street among human development just doesn't do anything for me, so I quit going outside. It seems like expulsion from the biosphere.
I wonder if other people feel this way, whether consciously or not.
[1] https://www.disappearingwest.org/