I mean, they’re already using LLMs. Namely, BERT.
There is no exact definition but BERT would probably just be a LM, not a "large" LM.
Is the exact definition important? The point is, they developed a thing and integrated into their core product. BERT allows them to handle conversational queries much better than before.
I think a Google Search Premium that cost $50/month would go over pretty poorly with Google's existing customer base (advertisers), but a startup can experiment with the business model with the right early adopters (e.g. Neeva).