Where the bottleneck is depends entirely on many details of the computations you wanted to run. IN many cases, you can get trivial embarassing parallelism if you can break your problem into N parts and there doesn't need to be any real communication between the processors running the distinct parts. In that case, memory bandwidth and clock rate are the bottleneck. but if you're running something like ML training with tight coupling, then the throughput and latency of the network can definitely be a problem.
If you want to play with it at home, connect those laptops to an ethernet network and install MPI on them both--you should be able to find tutorials with a little web searching. Then you could probably run Linpack if you felt like it, but if you wanted to learn a little more about how HPC applications actually work, you could write your own MPI application. I wrote an MPI raytracer in college; it's a relatively quick project and, again, you can probably find a tutorial for it online.
Edit: Your cluster is going to suck terribly in comparison to "real" supercomputers, but scientists frequently do build their own small-scale clusters for application development. The actual big machines like Sequoia are all batch-processing and must be scheduled in advance, so it's a lot easier (and cheaper, supercomputer time costs money) to test your application locally in real-time.
For actual computing a modern higher end processor/server will murder it but its' closer to the real world of clusters than anything (so much so that there is a company that does 100+ pi node clusters for super computing labs to test on, you can't obviously run scientific workloads but it's cheaper than using the real machine as well).
https://www.zdnet.com/article/raspberry-pi-supercomputer-los...
What software would one use to distribute some workload between these two nodes, what would the latency and bandwidth be bottlenecked by (the network connection?) and what other key statistics would be important in measuring exactly how this cheap $400 (used) set up compares to price/watt/flop performance for top 500 computers?