Heck, maybe it's time to go back to 55 as a federal limit. Last I checked, most vehicles on the road get dramatically better gas mileage at 55. Rather, it gets exponentially worse as speeds increase past 60ish due to wind resistance.
Hard limits are strange for things that are continuous and probabilistic. If we could set an automatic fee equivalent to the cost of increased risks, pollution, etc., it'd be a function of speed. Someday we'll have the technology to communicate that back to the driver as they change speed and location from urban to rural, go through construction zones, etc.
Of course, setting an appropriate gasoline tax, paid at the pump, would reduce the value of those fees.
Data doesn't back you up. In places where they have raised the speed limit, the overall flow speed does not increase correspondingly.
People drive at the speed they deem safe irrespective of the speed limit.