I’m a bit frustrated here, because physicists often seem to retreat to this position that it’s all just a question of terminology once people start pushing back against their philosophical claims. If Aaronson actually is using terms in such a weird way as you suggest, then I just have no idea what he is on about. We already have a perfectly fine word that means unpredictable; there’s no need to repurpose “free”.
I admit that I have no way of knowing what he has or hasn’t read, and my comment on that was snarky. But he doesn’t refer to any philosophical work in the interview, and I couldn’t find much published work by him that really engages with the current literature.
https://arxiv.org/abs/1306.0159
Scott is making a pair of claims: If it's possible to build a fast, noninvasive, perfect predictor then what more can science say to show that people don't have free will?
If it's impossible to build such a predictor, for some fundamental reason, then what more can science say to show that free will exists.
Before quantum mechanics and uncomputability, the "of course" went the other direction.
FWIW, I think Scott has read more of the philosophical literature on free will than probably anyone else in the world with a comparable level of quantum-physical expertise. If he's too confused to be allowed to discuss these issues, then what is the path by which philosophers expect to stay relevant and up-to-date with new knowledge? A field whose currency of legitimacy is "you must have devoted your life to understanding every detail of dispute in the existing literature" is not a living field that hopes to learn from outsiders and grow with new scientific inquiry. I think the best philosophers recognize this, and are willing to engage more broadly.