New York 500 Startups dude Shai Goldman has a good list going here: https://docs.google.com/spreadsheet/ccc?key=0ArI2sAC4lTszdGN...
If you're looking to use some independent data source that doesn't involve talking to people (which is the wrong way to go about it because fundraising is inherently a social networking exercise), I'm not sure all the data is universally public. The best source for brand new financings (although not follow-on rounds) is probably the Twitter bot VCDelta (twitter.com/vcdelta), since VCs tend to be good at updating their portfolio pages. Perhaps you could also get institutional fundraising information from the Form Ds (formds.com).
I suspect the Crunchbase data will only get worse as the importance of TechCrunch continues to shrink.
Even when you have the data though, it's hard to tell which investors are actually still doing deals. There are a lot of small funds out there that may not do a deal every 6 months even when they are still actively looking, perhaps because they are in the tail end of their investment period and are trying to be very selective, or perhaps because their typical bite size is large relative to the capital they have to deploy. There are also investors who will tell you that they are continuing to look at deals even when they aren't in a position to invest because they don't have committed capital and it doesn't look good to be out of the market. So all around it's a pretty fuzzy condition that you are looking to describe.
Of course, having a list is still nicer than not having a list, because if you simply "tap your network" for active funds, people will just think about who they've interacted with recently, rather than actually having any knowledge about the specific proclivities of the country's hundreds of venture capital firms, organized angels, etc. It's easy to overlook reasonable candidates.
Side Note: A little game theory... it's probably not a good idea to use a data source (crunchbase) that is heavily influenced by those who you are currently negotiating with. Sounds a little like back in 2007 when Goldman and Co were the ones rating the same junk securities they were trying to offload.
Entrepreneurs who just go by this instead of doing their own research (which really doesn't take that long) are doing themselves a massive disservice. Which is ironic, because this whole promotion was wrapped in a big bundle of 'rah rah, I'm helping entrepreneurs'. Not at all so.