The biggest problem visible on the TNG sets is the black cardboard pieces on the consoles in the rear of the bridge, used to block reflections from the lights. Those weren't visible after conversion to NTSC, but in HD they're noticeable. I'm not a director, but I wouldn't call this a problem with a shoddy set, but rather too many assumptions made at the time about how the video would be viewed. Surely, if they were filming a theatrical movie at the time instead of a TV show, they would have simply filmed it a different way, or rigged the lighting differently to avoid this problem.
That doesn't just meant that smaller details weren't important, so they were left out. But also that if something in your set needs to fulfill a role in the story, you better make that thing big enough to be legible on an NTSC screen, instead of something more subtle.