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Re:NixOS RFC 136 approved: A plan to stabilize the new CLI a... by chriswarbo on Sunday August 13, 2023 @11:47AM (#37111022)
These options got GUI icons to appear for me (on Manjaro, an Arch derivative):

  targets.genericLinux.enable = true;
  xdg.mime.enable = true;
  xdg.systemDirs.data =
    [ "${config.home.homeDirectory}/.nix-profile/share/applications" ];

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