That’s not a guarantee, of course, and it could be possible for police to corroborate that you had contact with someone else in another way (through records from a wireless carrier or by doing shoe leather investigative work) and use try to get data on that person to get them to testify, but if their only link was through messages that had been deemed inadmissible, they can’t use that witness.
The more likely question in a scenario you describe would be if the compromised Signal data would be enough to raise questions about the validity of all the data on the device. I.e., if Signal is out, can they use information from WhatsApp or iMessage or whatever. Past case law would suggest that once compromised, all of the evidence from the device is compromised — but a judge might rule otherwise.
It would be cool if Signal or another app could use those exploits they’ve uncovered to inject randomized data into the data stores of other messaging applications too. You know. Just as an experiment.
In the example being discussed here, it's absolutely still fine for LE and there isn't a need to find a secondary source that side-steps the FOTPT argument. In fact, I could drag a subject into an interview, take his phone and present a warrant to search his phone.
If he refuses to unlock the phone, I can say "fine, we'll use our special software instead" and take it back to another room. After the interview, I give him back his phone and immediately bring in his co-conspirator. If I show the conspirator fake messages between him and my first subject and get him to testify against my subject, that's still admissible. If this is the case, why would using potentially-false/unverifiable Cellebrite data be inadmissible?
For example, let's say they extract the Signal message data from your phone. You successfully convince everyone that this data might have been the result of some tampering. However, that doesn't prevent investigators from using that message history to find the other person, and get them to testify against you.